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The fullest analysis can only be achieved if rotational structure is resolved.
Rotational structure is, however, rarely resolved except for molecules with only two or three atoms.
This is quite enough to remove any resolvable rotational structure with the possible exception of sharp Q branches.
The title of Neko Case's new album, "Middle Cyclone," is a reference to "mesocyclone," the core rotational structure of a thunderstorm, which can produce a tornado.
In many cases, REMPI provides spectroscopic information that can be unavailable to single photon spectroscopic methods, for example rotational structure in molecules is easily seen with this technique.
Because the laser transitions are actually on vibration-rotation bands of a linear triatomic molecule, the rotational structure of the P and R bands can be selected by a tuning element in the laser cavity.
A rotational spectrum of the Π electronic ground state of l-CH can be made using the PGopher software (a Program for Simulating Rotational Structure, C. M. Western, University of Bristol, http://pgopher.chm.bris.ac.uk) and molecular constants extracted from the literature.